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10.1385/ct:5:3:257 16 BhuvanasundarR.JohnA.SulochanaK

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A recent computational study—using both DFT and ab initio methods—shows that there is a mixing between Co 4+ =O and Co 3+ –O • in a cobalt–oxo complex, with the former a breach of the oxo wall, and the extent of which can be tuned by varying the ligand architecture [67].) Metal–oxo complexes with the metal in a high oxidation state (as in Fe 4+ O and Mn 5+ O) cannot be stabilised by multiple bonding to an oxo ligand [63]